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    Bottom-up assembly of ultrathin sub-micron size metal-organic framework sheets

    Year: 2013

    Journal: DALTON TRANSACTIONS, Vol. 42, p 15931-15936, 20150722

    Authors: Makiura, Rie; Konovalov, Oleg

    Organizations: Osaka Prefecture Univ, Res Org 21 Century, Nanosci & Nanotechnol Res Ctr, Sakai, Osaka 5998570, Japan; Japan Sci & Technol Agcy, PRESTO, Saitama, Japan; Japan Sci & Technol Agcy, CREST, Saitama, Japan; European Synchrotron Radiat Facil, F-38043 Grenoble, France

    A solution-based two-dimensional interfacial reaction between 5,10,15,20-tetra(4-pyridyl)-porphinato zinc(II) (ZnTPyP, 1) and Cu(NO3)(2)center dot 3H(2)O, 2, results in the assembly of uniform preferentially oriented highly crystalline metal-organic framework nanosheets, NAFS-21 that have sub-micron planar size and mono-molecular thickness.