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    Omnidirectional Self-Assembly of Transparent Superoleophobic Nanotextures

    Year: 2017

    Journal: ACS Nano, Volume 11, JAN, page 587–596

    Authors: Wong, William S. Y.; Liu, Guanyu; Nasiri, Noushin; Hao, Chonglei; Wang, Zuankai; Tricoli, Antonio

    Organizations: Australian Research Council (ARC) Discovery Project [DP150101939]; DECRA [DE160100569]; Australian Microscopy and Microanalysis Research Facility (AMMRF); Australian National Fabrication Facility (ANFF)

    Keywords: omnidirectional scalable self-assembly; re-entrant textures; superoleophobic and superamphiphobic; ultra-transparent and flexible

    Engineering surface textures that are highly transparent and repel water, oil, and other low surface energy fluids can transform our interaction with wet environments. Despite extensive progress, current top-down methods are based on directional line-of sight fabrication mechanisms that are limited by scale and cannot be applied to highly uneven, curved, and enclosed surfaces, while bottom-up techniques often suffer from poor optical transparency. Here, we present an approach that enables the rapid, omnidirectional synthesis of flexible and up to 99.97% transparent superhydrophobic and -oleophobic textures on many variable surface types. These features are obtained by the spontaneous formation of a multi re-entrant morphology during the controlled self-assembly of nanoparticle aerosols. We also develop a mathematical model to explain and control the self-assembly dynamics, providing important insights for the rational engineering of functional materials. We envision that our findings represent a significant advance in imparting superoleophobicity and superamphiphobicity to a so-far inapplicable family of materials and geometries for multifunctional applications.
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