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Icephobic performance of one-step silicone-oil-infused slippery coatings: Effects of surface energy, oil and nanoparticle contents

Year: 2020

Journal: J. Colloid Interface Sci., Volume 558, JAN 15, page 251–258

Authors: Cui, Wenjuan; Pakkanen, Tapani A.

Organizations: University of Eastern Finland

Keywords: Lubricant-infused coating; One-step fabrication; Silicone oil content; Nanoparticle content; Ice adhesion; Freezing point; Surface energy

Hypothesis: State-of-the-art superhydrophobic surfaces (SHSs) usually do not function in high humidity and frosty climate conditions. Lubricant-infused slippery surfaces (LISSs) with a homogeneous and ultra slippery surface are expected to be a reliable icephobic technique. Hence, the fabrication of simple and scalable bioinspired LISSs is important for practical applications. Experiments: Durable one-step LISSs consisting of silicone oil and polymer mixtures were fabricated. A grid map based on added oil and silica nanoparticles was developed to tune wettability, morphology, and slippery behavior of surfaces. A similar framework for ice adhesion of lubricant-infused coatings was also presented for the design of optimal icephobic materials. Findings: LISSs with slight hydrophobicity yield slippery properties, resulting in an order of magnitude lower ice adhesion compared to SHSs. The stable 20-w% silicone-oil-infused slippery coating with slight hydrophobicity and silica nanoparticles was found to be effective in anti-icing. The nanoparticles firmly anchor the oil overlayer and eliminate contamination by drying the surface. The LISSs made of polymers with surface energy ranging from 29 to 31 mJ/m(2) show the potential to achieve low ice adhesion. As a result, the use of systematic frameworks highlights the role of material parameters. One-production strategy can be broadly used to design icephobic materials. (C) 2019 Elsevier Inc. All rights reserved.